LRTAP-4-76.pdf (3.043Mb)

CORRECTIONS ADDITIONS TO, AN~S OF LRT AP-DAT A

E FINAL REPOR OF TH

EC EMBER 197 4

JULY 1972 - D

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LRTAP - 4/76 DECEMBER 1976 ...

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~ I ADDITIONS TO, AND CORRECTIONS OF

THE FINAL REPORTS OF LRTAP-DATA, JULY 1972 - DECEMBER 1974

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l'JORv~EGIAf'l INSTITUTE FOR AIR RESEARCH P. BOX 130, 2001 LILLESTRØM

NORWAY

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INTRODUCTION

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Since the final reports were printed, a few errors and som misunderstandings have been discovered. Also some missing data are now available. The defects are briefly described on the following pages, and updated pages to be inserted in the original reports are included.

The name of the Dutch station NL 2 has been printed incorrect in the list of stations in the reports.

The correct name is Witteveen.

The aerosol sulphate data in the final reports of LRTAP- data (LRTAP 4/7 4, 4/75, 18/75, 19/75, 20/75, 2/76) from Austria, Germany, France and Iceland, are the figures reported to the CCU ("SO4XRF"-data) multiplied with 0.8.

As shortly described in LRTAP 4/72, this was done to correct for systematic errors in the X-ray fluorescence method, and to estimate the true air concentrations of particulate sulphate.

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It should be pointed out that this correction has not been applied to the aerosol sulphate data from Austria, Germany, France and Iceland in the three reports which give mean

concentration value and frequency distributions (LRTAP 12/75, 13/75, 3/76) .

Jan Schaug

~INAL REPORT OF LRTAP-DATA JULY - DECE~IBER 1972

7 July - December

The sulphate in precipitation data from the Finnish stations were corrected twice for seaspray.

July October

The particulate sulphate data from the Norwegian stations were missing in the report.

October

In October the station codes SO3, S04, S05 in the

particulate sulphate tables were interchanged cyclically.

The corrected data are given on the pages following.

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PREC!PITATfD SULPHATE (1-\ILLIIGRAMS PER M2)

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• LONG RANGE TRA-.iSPORT OF AI~ POLLUTANTS, FINAL ')ATA ^t1 AUGUST 1?.

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SULPHATE IN PRECIPITATIO~ <MILLIGRAMS PER LITEq), WHEN COR~ECTED FOR SEA-SPRAY MARKF.O WITH ASTERISKS

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DATE" N 23 N ?4 S 01

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'7 ~I~• POLLUTANTS•

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LONG RANGE TRAI\JSPORT OF FINAL )ATA AUGUST 72

StJLPHATE COLLECTED ON FI~~ER (MICROGRAMS PFR µ3)

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^{0.9 2,4} l. 6 35.0 27.5 20,0 3.0

1.a

0. 6 3.9 1 • 6 13.0 15 o.o o.o 3.2 2.8 O.A 0.1 1. 3 10.0 10.0 17.5 10.0 3.0 3.1 4.8 1. 9 7.0 16 o.o o.o 2.3 1.3 l • l 1.3 3.4 7.5 3.0 17,5 3.1 3.1

2.s

s.o 3.?. 11.0 17 l ^O l♦

o.o

0.1 0.6 1.2 5.1 3.0 20.0 17.5 12.s 4.7 il. 5 l. 1 A.7 3.3 5.0 18 0.7

o.o

o.o 0.3 0. 1 O.il 0.2 2.5 15.o 2.5 1.0 1.8 o.o 20.3 l. 5 4.0 19 1.9 o.o o.o o.3 0.1 0.1 0,6 2,5 o.o 2,5 l. 1 0.5 0,2 A.7 0.3 ^A00

?O 1.0 o.o 0.3 0.1 0.1 1.7 0.9 20.0 7.5 15.0 1.2 1

.a.

^{o.o A.8 l • 1 5.0}

21 1.7 o.o 0.1 0.6 2.2 0.4 2.5 ?. ^e 5

2.s

1,3 o.o 9.1 0.4 4,0 22 2.2 0.1 0,5 0.1 2.2 o.e 2.5 ?.c; 2.5 1.6 0 .5 0,4 1, 9 0.4 9.0 23 o.s o.o o.4 0.6 o.o 1.8 o.3 7.5 ?.5 5,0 0. 6 0.2 0.4 4.6 0 • 6 24 2.6

o.o

0.2 0.2 0.1 0.1 0.i i O ^a 0 2. c; 2.5 0.1 0.1 o.o 2.3 O.B 11 .o

?5 o.s o.o o.o 0.3 0.1 0.9 o.5

s.o

2.5 5.0 o.o 0,4 0.1 l • 2 1. 4 12.0 26 0.1 0.3 l • l 1.4 1 .4 0.1 2.5 7.5 2.5 o.o 0.1 0.4 2.6 1.3 2.0 27 1.4 1.4 l. l 0.4 0.2 1.0 1.2 7.5 10.0 7.5 0.1 0.8 1. l 2.9 2.1 2.0 28 4.3 l • 5 2.1 2.3 0.1 3.4 12.5 10.0 7.5 0.2 o.o l. 7 ?.7 1.3 s.o

. I

^{2') 1.0 1.0 1 •}

^'°

^{3.1 l • 1} 3.3 0.6 15.0 12.s 10.0 1. 9 2.0 0.5 2.2 0.4 6.0 30 o.s 2.4 2.1 2.7 3.2 2.3 o.a 17.5 10. 0 12,5 l • 6 o.5 1.0 o.6 0.3 5.0 31

o.o

2.8 4.8 17.R 3.0 2.a 1 .4 7.5 10.0 10.0 l. 9 1.7

o.s

3.4 1.0 6.0

,w.J

J

J

J

J

J

J

7

7

LONG RANGE TRA>.JSPORT Of Al~• POLLUTANTS, FINAL ')ATA ti1Jr,usr 72

PRECJPITATfD SULPHATE (MILLcrGRAMS PER M2)

7

^{DATE JC} N 01 N 03 N 05 N 06 N 07 N 08 N 09 N 10 Ill 14 N 15 N 16 N 17 N 18 N 19 N ?.O N 21 N 22

1 13 13 9 5 9 4 4 s 1 3 25 19 20 17

2 20 2 11 40

3 3 2 16 11 4 10 35

r

1

^{5 4 37 44 18 4S 63 46 33 0 30 2 1 6 8 26 29 19 19 4 10 9 229 117}

6 68 109 34 34 59 106 11 1 85 8 2 13 53 10 38 ⁹³

7 100 32 90 18 49 51 41 45 9 )9 66 40 54 67Q 88 84 !6~

1

A 69 ¹⁰⁷ 66 68 1S6 99 43

sa

4 24 ^{38 100} 88 115 37 44 159

9 9 19 9 20 14 4 3 24 2 20 70

I 0 2 11 5 10 7 1 2 2 5

11 3 I 4 I 0 l 0 0 0

12 6 0

. l

^{13 33 34 22 52 24 19}

14 2 3S 29 136 69 7 7 25 40 5 63 37 34 33 260

1s 3 s 16 28 77 s s

~ l

^{16 17 5 8 8 11 1 3 2S 5 49 l 11 l 33 6 6 ? 3 0 2 28 l 13 4 20 16 1 11 7 21 18}

18 I 0 0 0 3 2

19 11 0 0

20 ₆ 0

. I

^{21 1}

22 ^{. 0}

23 0 0 7 0 2 4 1 3 2 ³ 7

24 l 0 0 1

25 1 0

26 1 0

27 7 0

28 67

29 4

30 3 3

31 13 ₂

PRECIPITATED SULPHATE (MILL'lGRAMS PER "12)

DATE N 23 N 24 S 01

s

04 S 05 SF SF 2 SF 3 SF 4 SF 5 Ut< l

1 241 3 22 55 ~

-

9 181

_j

^{2 3 4 80 14 19 4 100 43 14 4 37 7 15 3 52} 8 1 l

5 6 9 21 21 27

6 14 68 ² 5 ^Q 0

_J

⁷ ₈ ^14~ _{47 34} ¹⁸

9 41 36 14 5 1 0 70

10 29

J

^{l 1 12 13 16 4 59 42 13 99 9 3 10 2}

J

^{14 15 16} ₁₇ ³⁵ ₁₈ ²⁶ ₁ 44 ^{26 13 14} 4 ^{9 12 30 53 91 48 15 41 11} 14 ⁴

18 40 4 83 so 23

J

^{19 20 4 1 42 2 I 8 2 9}

21 13 127 14 37

22 3 3 26 63 17

J

^{23 24 25 2 4 17 5 0 4 2 25 2 ';i s 78 25 32 3 5 9 5}

26 5 5

J

^{27 28} 29 ^{0 28 6 12 l 0} s

30

J

^JI

7

7

, LONG RANGE TRA~SPORT OF Al~· POLLUTANTS• FINAL ')AJA i «:;EP TEMAER 72

SULPHATE" IN PRECIPITATIO~ (MILLIGRAMS PER LITER>. wHFN CORQECTED FOR SEA-SPRAY MARKFD WITH ASTERISKS

7

^{l)ATE N 00 21 N}

^••

22 Ill 23 N 24 ^{00 00} s ⁰¹

s

⁰²

s

⁰³

s

^{04 S 05 SF}

^•

^{l S• 2}

^•

^{SF 0 3 SF}

^•

^{4 c;F 0 5 UK 1 0}

1 1.1

~ l

^{2 3} 4 ^2,8 0,4 ^{o.o p.o 6.3 ;;> ,q} 0.1 ^{2.1 ?,0} o.5 ^{6.2 1.5} 1 • !t· ^{1.8 0.9}

5 2.4 o.o 1.5

6 1.5

-

^{12.3 19.l 0.9}

~ l

^{7 9,3 1.5 8.6 21.2 7.6}

8 0.1 1.2 12.0 1.2 c:; • l 17.l l O.? 10.1+ 2.9 5.q

9 l. I'> l0o3 l 0, 4 l. 3 1.2 i:,• l n. 2 o.,c,

10 0.3 3.5 1.? 5.0 5.0 ;>. 7 ?.4

~ l

^{1 l 12 1.3 0.2 0.4 o.5 2.9 2.6 2. 1 10.? A ,4 4.0}

13 2.2 1.5

a.a

^{2. c:;}

14 1.6 5.2 1.2 0.9 70A 5.0

15 2.4 l • 6 B.3 o.o 5.2

16 8.3 3.2 1.i:i 8,3 o.o 2.0

17 8,3 o.o 0.6 4. l

18 0.9 1. 9

19

20 6.1 6.9 2.3 l. 1

21 6.7 1.4 5.0 6,9 4.7 3.9 3.6 1.5

22

o.a

^{e.5 3oA 5.7 2.0 1.2}

?3 2.6 3.1 1. 5

?4 1.5 o.o

25

a.a

0.6

26 5.0 2.3 2.4 1.8 0,8 2.1

'21 6.4 1.5 2.3 2.1

28 1.7

29 30

PH IN PRECIPITATION_-

DATE D 01 JC 1 N 01 N 03 N 05 N 06 N 07 N 08 N 09 N 10 N 14 N 15 N 16 N 17 Ill 18 N 19 N 2(1 N 21

1 6050 5.35

2 6.20 5.00 '5.30

3 5.20 6025 5,35

4 s.oo '5,90 5.70

J

^{5 5.10} 5,50 5,45

6 4,40 4.55 6.25 6. 15 4,85 4.70 5,?5 4.80 4,80 6.15

7 3.80 3.95 6.50 4. 10 6.05 4,15 4.05 3,95 4,50 4.25 4.15 3.85 4 • 1 'i 3. "95

A 6,20 5.50 6,35 5,45 4o 15 6.10

I

^{9 4.20} 4.05 4,10 4,20 5.20 4. 10 4,c;S 4.7c; tt.40 5,05 4.60 4o25 4.05 4,15 s.q5 4,40 4.60

10 4o20 6,45

-J 11 4.30 5.c;o 6,30 6,60 5.50 6.05 5,75 4,50 6.30

12 4.40 S,AO 6,50 7,00 6,20 6.30 5,65

-

^5.80

13 4.40 3.60 6,10 6,05 5.70 5.10

_j

^{14 6,30 5,95 l',,40} 6,95 4,80 4,90

15 4.40 5,QO 5,55 6.50 4,70 5.45 5,lo

16 4.50 6,20 4,85 5.05 5.10 5,55 4.65 4.80 5,60 4,95

J

¹⁷ 4.20 6.oo 6,65 6060 6,45 5,90

18 5,00 6,00 5,45

19 5.60 5,65

20 5.70 5,60 5.35

J

^{21 5.90 3.85} 3.65 3.60 4.50 4,30 5,50 5.30 4.25 4,00 4,65 4.40 4,40

22 4,20 6.00 5.95 6,85 6.10 5.20 5.75 5,1',0 5,70

23 5.10 6,55 6,20

24 4.60

25 6.20 5,80 5.30 6.05

J

^?.6 4.10 4,90 f,,35 n,oo 5 .12

27 6,60

28 5,40 5,45

J

²⁹ 4.20 6.00 I',, 15

30 5oAO

7

7

LONG RANGE TRANSPORT OF Al~ POLLUTANTS, FINAL )ATA <;EPTE~AER 72

S02 IN AIR ( MICROGRAMS :,ER: M3>

.. 1 DATE s 04

s

05 SF 2 SF 5 U'< l

l 25 0 10 11 3

2 27 0 14 0 0

3 27 0 12 8 0

4 33 0 15 l 0 2

5 48 0 27 7 0

6 32 0 30 9 11

7 26 0 18 8 15

8 28 0 27 0 20

g 30 0 18 0 15

10 23 0 19 0 28

11 2,. 0 16 13 8

12 25 0 34 15 43

. l

^{13 35 0 8 0 12}

14 ¹⁹ 0 13 0 7

15 0 0 18 0 16

16 0 26 13 0 53

17 0 3 0 0 22

18 0 0 11 5 7

19 ⁴ 30 5 7 10

20 ⁰ 0 36 5 30

• I

0 30 40 5 21 21

22 ⁰ 0 13 5 32

23 0 20 5 5 5

?4 0 0 8 9 5

25 0 17 5

26 0 32 15 43

2~ ^{0 4} 17 43

28 0 0 6 29

29 0 29 10 89

30 ^{0 23} 5 31

SULPHATE COLLECTED ON FILIER (MICROGRAMS PER M3)

DATE TC l N 01 N 03 N 09 N 21 N 22 N 23 NL l NL· 2 NL 3 s 03

s

⁰⁴

s

05 SF 2 SF 'i UK l l o.5 4. 3 8.4 4 .• 8 7.3 1.1 10.0 10.0 2. 4 3.0 2.2 3.7 2.0 A.O

- l

^{2 0. ;> 5.6 6.A o.s 5.1 2.5} 1. 5 12.5 10.0 4.B 1.3 o.o 2.5 0. 4 10.0 3 0.2 0.1 0.2 o.s 0.2 2.0 o.5 30.0 17.5 1 • 6 1.a 0.2 2. 3 0.1 R.O 4 1.2 0.3 0.3 l • 6 o.s o_.a 0.6 5.0 2.s 12.5 o.o o.o 0.2 0.6 o.o 3.0

J

^{c; l.? 0.0 1.7 2.1 1.4 2.0 0.1 7.5 2.c; 2.5 1.9 l • l 0.1} 3.2 0.2 6.0

6 0.1 l. 7 4. 3 6.7 1.3 5.8 1.2 32.S 30.0 10.0 4.6 2.4 6.5 __ 7.8 1. 5 22.0 7 o.5 B.3 4 .6 0.2 ei. 3 15.2 7.6 77.5 50.0 40 • 0 15.5 g. 1 7.6 6.2 3.7 11.0 A o.5 0.2 0.1 0.5 o.o l. 2 0.3 32.5 20.0 15.0 5.0 10.0 2.2 23.4 11.3 a.o

J

^{g o.s 3.4 1.8 0.1 o.5 9.7} A.7 30.0 22.5 12.s 12.a 7.1 1. 9 3.9 2.4 5.0 10 0.2 0.2 0.'3 0.2 0.2 o.5 0.2 5.0 2.c; 2.5 4.6 12.s 2.s 17.0 3.3 3.0 11 o.o 0.2 0.5 o.o 0.1 0.1 o.3 15.0 5.0 7.5 o.o 2.8 0.4 11.0 11.5 2.0 12 0.2 0.1 0.3 o.o 0.1 0 • 9 0.1 12.5 10.0 5.0 o.s 1.0 0.4 2.1 12.1 f,. 0 13 0.5 0.3 0. 1 0.3 0,3 2.0 n.5 17.5 7. r:::, 7,5 1.0 o.s 0.2 1.6 1.7 3,0

J

^{14 0,2 0.6 0.1 0. 2· 0.1 2.7 0.8 15.0} 7.5 2.5 1.8 1. 3 0,5 3.4 2.6 2.0 15 0.1 0.4 0.5 0.3 0.6 1.3 0.7 2. 5 o.o 2.5 1. 6 3 .• 1 0.7 17.4 l. 4 6.0 16 0.1 0.1 1.7 4.2 7.5 4.9 l • q 2.s o.o 2.s 0.1 10.2 1 • 1 ^16.9 2.7 9.0

J

^{17 o.? 4.7 4. 0 6.2 6.8 6.9} P..7 10.0 ^1.c; s.o 3.1 3.4 o.s A.3 0.7 s.o 1 A 1.4 2.9 5.4 l. 9 1,7 3.1 2.2 15,0 5.0 7.5 0. 4, 0.2 o.o 1 ~ 1 0.6 4.0 19 l. 4 4.6 ^4.4 0.4 1.3 8.2 6.9 37.5 15.0 17.5 7.8 0.7 . 0. 0 0.8 _{1 • 1} 15.0

;>O 0,7 3.0 6.6 4.R 3.0 12,9 3.2 27,5 15.n 22.5 4.3 4.6 0.1 2.7 l • 6 18.0

J

^{?.l ?2 0.?. 0,7 4.9 0.5 0.1 0.2 0. 0.2 f, 2.2 0. l o.o 0.4 p,.} 0.2 42.'i 20.n 20.0 ^{1 30.0 21.c; 15.0 6.9} o.o ^7.6 l • 9 ^{0.5 10.9} o.o 5.3 ^{2.6 10.0} 3.0 21.0

?l 1.4 0. l 0. l 0.1 0.2 0.6 0. l 2.5 2.5 2.5 0.1 o.o o.o I • 1 O.A 6.0

?4 ?,9 0. l 0.2 0.9 0.4 0.1 n.2 ?,5 o.o 2.5 0.2 0.4 0.4 1.7 1.0 1.0

?5 A.2 J.5 l • l 2.1 0,6 2.5 2.2 5,0 ?.c; ?. • 5 l • 1 l • 1 0.5 14.7 0.6

J

^{?f, 4,1 0,6 I. 0 I • 0 0.8 3.8 I • 7 s.o s.o 7.5 0,7} 0.4 0 .-o · 6- • .3 1.4 10.0

?7 0,5 0.6 0.7 O.R 0.2 0.6 0. r, 7.5 s.o 5,0 o.o 0.4 0.4 1.5 10.5 H,.O

?A 0.1 0,8 1.1 1.9 0.2 1.3 o.5 5.0 ? • c; o.o 0.2 0.2 0.2 4,8 o.o 16.0

_j

^{?9 0,5 1. 3 l. 2 0.5 0.6 2.0 3.0 7.5} ?.5 12. 5 0. l 1 • l 0.1 1.2 3. 9 21.0·

30 0.5 1). 6 o.o 0. I 1,5 1.5 1.6 17.5 1.c; ?.7,5 0,7 1.B o.c; 1,8 2.0 15.0

7

7

LONG RANGF TRANSPORT Of AIR• POLLUTANTS, FINAL :)ATA <;EPTE~AER 72

PRECIPITATED SULPHATE (~ILL1GRA~S PER M2l

7

DATE IC l N 01 N 03 N 05 N 06 N 07 N 08 N 09 N 10 N 14 N 15 N 16 N 17 N 18 N 19 N 20 N 21 N 22

l ⁾

2 8 7

3 53 ?.

4 68 l

5 1 l l 1

6 9 8 4 5 3 19 19 4 10 11 2

. I

^{7 8} ₉

_-

_{452 339} ¹⁴ ₃₃₀ ^{3 29} ₉₀ ² ₁₇₄ ^{4 62} ₅₇ ^{3 102} ₃₉ ¹ ₁₈₅ ^{12 21} ₇ ^{1 23} ₁₆ ² ₈₀ ^{14 1} _{219 137} ¹³ _{288 34} ^{6 33} _{53 207}

^-

JO 1

11 6 2 2 l l 9

. l

¹² 13 ^{6 l 1} 0 ⁰ l ⁰ 1 ^s 4 ^I A

14 8 l 0 10 16

15 l 0 26 24 20 l 32

.

⁾ _{16 l 14 13 35 6 26 35 18 9 22}

17 1 2 5 0 0

18 l 0 l

19 19 0 l

. I

^?.0 ₂₁ ² _{l 24} 43 67 37 77 ² 9 ² 1 7 11 16 4 16

22 27 0 5 1 2 8 2 0

23 24 1 0

24 25

?5 0

-

^{4 3 2}

?6 3 l 0 l 13

21 2

28 6 0 1

?.9 15 0 lo 0

30 3

&

I

PRECIPITATED SULPHATE (MILLIIGRAMS PER M2)

DATE N 23 N ?4

s

01 s 03

s

⁰⁴

s

^{05 SF} Sf 2 ,SF" 3 SF 4 Sf 5 UK l

l 10 7

J

^{2 3 4 14 1 18 16 l A 2 3 16 6 9 I+ 5.}

^..

5 16

-.

⁴

J

^{6 7} 8 ^{5 A6 53} 4 ^{60 104} 54 2 15 47 12 26 ¹ 65

9 366 36 67

-

^{9 0}

10 4 42 179 28 62 24

11 2 8 9 16 26 ?.8

.. J 12 2 14 8

l3 1 33

J

^{14 15 16 24 9 5 23 31 22 17 ½ 20 78}

17

-

'

-

^{3 12}

J

^{18 20 19 62 3 2 3 15}

21 29 60 11 31 9 6·

J

^{22 ?3 ?4} _?5 ^{2 3 3 17 4 30}

^-

^{17 10 7} ₂

?6 2 3 A 4 1

J

^{?7 2A} _?9 ^{87 5 20 5 3}

.10

-1

rl

_QNG RANGE 1RANSPORT OF AJ~ POLLUTANTS, FINAL ~ATA OCTOBED 72

SULPHATE IN PRECIPIHTIO\J (MILLIGRAMS PER LlTf~>, WHFN CORRECTED FOR SEA-SPRAY MARKED WITH ASTERISKS

I .. .. .. .. ..

ⁱⁱ

DATE

s

⁰¹ s ⁰²

s

⁰³

s

⁰⁴

s

⁰⁵

s

⁰⁶

s

⁰⁷

s

^{OR SF 1 <;F 2 SF 3} SF 4 SF ⁵ UK 1 1

r I 2

3 o.o

4 2.1 1 • Fl 4.1

5

f,

-

^{21.3 1.1 1. 3}

r

l

_{7 21.3}

A 21.3 9.9

9 2.1 12.3

10 0.3 10.3

11 7.6 5.0 o.o 2.2 6.9 3.3

12 2.3 4.8 3.9 1.2

13 14

15 1.3 0.5 5.7

16 o.o o.o

17 o.o 5.3 1.0 0.4 o.o

18 11.0 lo 7 o.o 5.9 1.2

19 4.9 1 1 • 0 o.o 1.2 3.7 0.6 o.o 4.A o.o

20 2.4 1.0 o.o 1.9 1 • ?. 0.6

'21 2.4 2.3 1.4 4,4 o.o

22 2.4 o.o o.o 0.1 4.1 2. f,

23 4.8 o.o o.o 1. 7 10.0 l • l 0.9

?4 9.3 0.9 2.3 0.5 o.s

25 o.o 2.3 1.6 ?.3 o.s

?6 4.0 1.5 0.6 1.3

n

^22.0

2A 14.8 22.0 11.0

'29

-

^{22.0 _, 7.9 17.4 8. l l?.9 7.3}

30 2.0 3.9 8.7 6.5 2.5 6.6

31 5.3 1.2 ?.1 3.f, 4.7

tH

IN Ø-~ECIPITATION.

DATE 0 01 IC 1 N 01 N 03 N 05 N 06 N 07 N OB N 09 N 10 N 14 N 15 N 16 N 17 N 1 A N 19 N 2/1. N 21 N 22 N 23

l

-

2 s.90

3 4.20 4.50 6.45

4 5.AO 4.15 3'.45 4.10 4.90 5.35 6.20 4.35 4.30 3.70

5 4,90 5.B5 5.95 s.20

6 6.30 7.15

-

^7.15

^-

^s.20 5.05 4.55

-

L J

7 s:60 ,.75 6.40 -~

8 6.20 5.4;>

-

4.35 6.55

9 6,70 5.65 4.35 6040 6.15

-

_J

^{10 6.70} 3.95 3.90 4.85 4.95 4.35 4 • 10 6.20 6,45

11 5.90 6.55 3.5A

-

6.'25 4.Bo 1;.05

-

4.80 4.15 s.6s 6.35

-

12 6. l 0 5.55

-

_j

^{13 6.20} 5.70 S.85

14 5.60

-

5.85 4.80

15 6.40 <;.45 5.05

16 5.55 s.o5 5.35

-

17 . s.20

-

^6.55 5.40 5.30 6.75

-

J

^{18 6.25}

^-

5.75 5.55 s.2s 5.45

-

19 4.40

-

^{6.95 6.40} 5.55 6.00

20 4.20

-

^5.40

^-

J

²¹ ₂₂ ^{4.30 S.40}

^-

6.10 s.10 6.10 5.60 5.45 5.FlO f,.65

-

4.~s 4.00 5.7'-

- ^s.os

4 .4-0 5.25 4.80 5.70 4.85 5.55 5.AO 5.SS 5.?.0 6.30 c;. 1 5 5.50 6.A0

-

5.40 4,80 5.50 23 4.2Ø 4.90 5.25 5.25 6,35 6.60 s.65 5.70 S.3c; 5 • fiO S.95 5.30 6.25

24 6.Q0 s.75 6.00

s.1s

^5.45 s.65 s.10

25 4.20 6.90

-

^5.90 6.20 s.1s 4.65 4.65 6.05 s.10

J

^{';)f, 27 5.40 4.50 f,.60}

^-

^{3.90 6.ns 3.50}

^-

^3.~-

?8 6.30 3.80 3.90 3.90 3,65 4.no 4.30 4.()0 4.20 3.75 3.75 3.95

29 6.50 3.90 4.00 5.Bs

-

4.10 4.30 4. 15 3.95

-

^4olS

-

4.20 3·.A5

s.oo

10 4.30 4.15 4.25 4.45 4.15 4.30 4.75 4.10 4.35 4,.90 3.PO 4.00 1.i:.o 4.35 3.AO 4.}0

31 6.JO 4.35 4. c;c; 5.90 4.49 I+• 70 I'.. 00 6.85 4,50

7

LONG RANGE TRANSPORT OF ^A I~, POLLUTANTS• FINAL ')ATA OCTOREP 1?

7

S02 IN AIR ( MICROGRAMS ^::>f~ M3)

DATES 01

s

⁰²

s

⁰³

s

^Ol+

s

05 s 06 s 07

s

08 SF 1 SF 2 sr:- 3 SF 4 SF 5 UK l

r

l

^{2 1 13 4 0 0 0 0 0 0 13 0 122 18 8 70 47 13 5 26 17}

3 0 0 0 0 0 23 21 8 15 10 31

4 2c; 0 0 0 24 15 42 0 11 7 36

5 0 0 0 0 0 13 18 0 10 7 23

. l

^{6 0 0 0 0 0 15 32 0 0 5 33}

7 0 0 ⁰ 55 0 8 16 0 0 5 41

8 0 0 0 0 0 23 24 0 11 10 17

9 0 0 0 0 9 15 16 0 0 6 17

10 0 0 0 0 0 18 37 ^p. 12 0 18

11 0 0 0 0 0 16 17 16 0 0 15

12 0 0 0 0 0 16 14 l fi 0 0

13 3? ⁰ 0 0 0 8 13 ^p. 0 5 4

. l

^{14 0 0 0 0 0 0 11 0 0 0}

15 0 0 ⁰ 0 0 0 5 0 0 0 9

16 0 0 0 0 ⁰ 24. 31 30 15 15 3

17 0 0 0 0 0 0 15 8 26 15 17 5

l 18 0 0 0 0 0 0 0 28 5 33 17 17 7

}9 ₀ 0 0 0 0 0 0 33 0 27 13 16 3

20 0 0 0 0 0 0 0 33 0 2R 13 14 3

21 0 0 0 0 0 0 0 28 0 2~ 13 15 25

22 0 0 ⁰ 0 0 0 72 15 0 20 11 15 12

23 0 0 0 0 0 0 8 10 12 0 15 35

?4 0 0 0 0 0 0 0 0 11 10 0 0 16 36

25 0 0 0 0 0 0 0 0 10 16 0 0 10 40

?6 0 0 0 0 0 0 0 0 0 13 0 0 0 60

?.7 0 0 0 0 0 0 0 0 11 8 7 0 0 31

28 0 0 0 0 0 0 0 0 Ji• 16 0 0 0 27

29 0 0 0 22 0 0 104 0 15 11 0 0 0 15

30 0 0 0 22 0 0 0 0 8 16 11 7 7 35

31 0 0 0 22 0 0 0 0 8 28 1 0 2 59

SULPHATE COLLECTED ON FIL!TER (MICROGRAMS PF:R "13)

DATE OK 1 DK 2 DK 3 DK 5 DK 6 IC l N 01 N 03 N 0Q N 21 N 22 Ill 23 NL l NL 2 NL 3 s 03 s 04

s

os

j

^{l 1.0 lo3 1. 5 0.1 2.0} 3.2 2.3 22.5 15.8 25.A 2.6 2.3 9. 0

2 0.1 2.4 2.5 0.4 1.9 10. I+ 6.1 19.2 17.5 20.8 3.4 4.3 14.A 3 0.7 4.4 3.5 l • 1 3.4 12.6 0.2 15.0 12.s 1s.o f,. 1 A.1 9.6

4 0.2 11.4 9.3 0.2 3.1 ?7.6 7.3 16 • 6 15.8 20.R 13.2 7. 8 1 • 1

5 0.?. 0.7 B.8

o.o

0.3 13.0 1.2

-

^{21.6 17.5 13.0 7.A 0.1}

J

^{6 o.s 1. 5 0.4 0.7 0.3 2.9}

^-

35.0 56.6 63.3 A.O ?.9 2.0

7 o.5 6.6 26.2 o.o o.s 43.8 0.1 38.3 45.8 :n.s lP..7 5.3 s.a

A 0.2 1 7. 1 9.7 2?.s 5.8 61.4 o.o 24.2 44.l 21.6 18.7 22.2 6.7 9 0.2 3.6 33.4 17.9 4.0 54.6

-

21.s ?.5.0 14.1 16.0 22. 1 1.2

J

¹⁰ o.o n.o 1 5. 1 11. fi 8.9 49.9 ?4.A s5.a 29. 1 2s.o 11.7 19.6 4.7

11 0.2 6.2 0.1 0.4 o.J l 1 • O 6.8 25.0 17.S 11.6 6.6 6.9 o.a

12 o.s 0.3 0.2 0.1 0.2 1.0 0.4 7.5 ?.5 1.6 o.a 4.4 1.1

J 3 1 • 2 1.2 0.4 I • 0 o.5 7.6 3.9 3.3

o.a

0.8 a.o 10.8 l .2

J

^{)4 1.0 0.8 0. l l • 0 0.1} 9.7 2.6 11.7 10.0 6.6 s.6 7.Q 1.3

15 1. 2 0.1 0.2 1.c; 0.5 1.7 o.6 9.?. 4.6 2.s 1.9 1.9 006

16 o.s 0 .f> 0.2 1.7 o.3 3.3 1 • 1 3.3 5.0 3.3 1.7 2.3 o.6

17 1.2 0.3 o.o 0.3 0, 1 0.8 0.4 12.c; 5.0 3.3 o.a l. 1 o.6

J

^{?0 I A 19 0.1 1.4 1.s 0.2 0.4 0.1 o.o o.s o.o n.a o.o 0.1 0.2 0.9 0.1 0.1 0.3 0.4 0.3 0.3 0 • I 3.3 4. 2.s f, ?.. 5 1.6 0.8 o.o o.a 0.8 0.9 o.6 0.1 1.9 2.0 1.4}

^o.o

^{1.0 1 • 1}

?. l 1. 5 0. I o.3 2,6 0. l 0.2 0.4 2.5 o.o 0.A 1.3 1.n o.a

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?5 o.o 1.9 o.3

o.a

0. 1 4.5 1.9 18.3 12.s 6.6 2.0 2.6 0.1

J

^{?6 0.5} ?.5 2.2 2,6 0.4 18.7 3.5 20.A 19.l 13.1 5.9 1.0 o.s

?7 o.o Jg.6 14.0 7.? 3.3 I 5. !+ ?5.4 11.7 10.0 6. f, 15.2 2 .6 1.3

?A 0.?. q_7 I 3. 1 1 I • 6 4.2 ]9.f> 13.l 10,8 4.6 s.o 17.4 13.2 2.2

;,q o.o 10.0 0.9 -:,. • 7 0.1 }4.7 4,5 9.2 l I .6 s.a 9.6 12.1 2.5 10 7. I 11. 9 1.A 0.2 1.9 3.0 0.0 0.9 14.0 ^4,7 20.A 14.1 B.3 7.1 5.4 o.a 11 o.s 1.4 20.8 0.1 9.6 0.2 1.2 1,2

s.o

1. 2 11. 7 1.3 27.S 19.l I 1. 6 9.0 5.4 1.2

1

7

• LONG RANGE TRANSPORT OF AIR POLLUTANTS, FINAL DATA• OCTOBER 72 SULPHATE COLLECTED ON FILTER <MICROGRAMS PER M31

...,

_{DATE SF l SF} 2 SF 3 SF 4 S• 5 UK 1

l 3.7 1.6 14.0

2 1.6 5.1 3.6 1.9 1. 2 16.0 3 10.s 6.0 4.3 6.2 9.1 13.0 4 11.!l 9.7 8.5

s.o

2.8 ^16.0

r

1

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.. ·1 ^{8 ?7.1 6.9 3.3 6.7 0.8 8.0}

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-l

¹³ ₁₄ ^1.1 6. g ^7.9 5.8 ^4,7 3.4 ^{9,6 10.4} 6. 7 12.3 ^1.0 1.0 15 ^{I. 8 2.1 l. 5 1.6 1.5 1.0} 16 1. 0 12.8 1.0 0.6 0.5 1.0

• l

^{17 1.3 l. 6 0.4 0,3 o.5 4.0}

18 ^{1.3 o.s 0.9 0.9} loO 2.0 19 l. 9 1.8 2.a 2.2 l. l 1.0 20 2.5 2.6 406 3.0 0.9 4. 0

. l

²¹ ₂₂ ^0,7 1.8 2.2 14.5 ^{8.3 4.1 3o2} 9,7 ^2.1 1.5 4.0

^s.o

23 ^1.3 6.4 11 • 1 1.0 6.7 3,0 24 3.7 3.2 2.9 0.1 6.5 5.0 25 l. 3 2.6 l. 3 0.8 3.4 8.0

·26

1.s

2.9 Oo7 0.1 l. l 12.0 27 ^{4.8 3.8} 1.1 0,9 0.6 s.o 28 ^{21.0 2.7 3.0 2.s 0.6 3.0} 29 ^{9.9 5.4 1.0}

s.s

1.1 3.0 30 1o2 3.3

J.o

1.4 1.6 6,0 31

s.s

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. l

I I

~ I

J J J J J

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7

7

LONG RANGE TRA~SPORT Of AI~ POLLUTANTS, FINAL '.>ATA • OCTOAER 7?

PRECIPITATED SULPHATE <~ILL1GRAMS PER M2l

r

I

^{DATE IC} N 01 N 03 N 05 N 06 N 07 N 08 N 09 N 10 N ]4 N 15 N 16 N 17 N lfl N 19 N ?O N 21 N 2?

1

2 ^]

] c:;2 31 2

rl

^{4 5 10 1 2 22 30 14 16 l 3 2 4 2 4}

6 3 4 2 ^Q 9

7 ?

:v.

8 1 2 11+ 2

Q 3 4 13 2 6

10 27 ?9 ?.3 3 11 3 2 ^c;

11 3 7 1 9 1 17 43 4 77

12 1

. 1

^{13 4 l}

14 1 6

15 5 I+

'"I

¹⁶ 17 82 ⁸ 0 ² 4 ^I+ 3

I ^{18 3 2 B 4}

19 1 0 I+

20 l

21 5 3 0 0 5 l 10 n2 2

22 9 4 2 6 8 4 5 l 2 16 3 2 19

23 4 l 1 l 38 3 9 11 1 4 l 2

24 44 8 0 2 5 l l

?5 1 3 4 3 22 35 3

26 5 1 3

?7 3· 6 13 30

28 64 32 66 35 39 ?3 2A 12 19 21

29 0 31 38 15 19 42 78 9 10 2 33

• l 30 27 24 23 23 18 36 4 6 11 8 5 2A

31 8 15 7 18 0 7

PRECT'PITATED SULPHATE (~ILLIGRAMS PEQ M2)

DATE N 23 N 24

s

01

s

03

s

⁰⁴

s

⁰⁵

s

06

s

07

s

OA Sf SF 2 Sf 3 Sf 4 SF 5 UK 1

2

.. I

⁴ 3

_s

₆ ⁹ ₀ ³ .;.

-- -

^{6 2 14 2}

J

^{7 8} _{9 3} ⁶ _{2 25}

10 121 l 31

_l

^{I l 12 91 18 6 9 6 37 14 f,8 ]4}

13 3

J

^{14 15 16} 17 ¹⁹ 2 12 ¹⁰ 1 ^?6

l 8 3 9 c; 2

J

^{20 )9 3 15 7 5 4 1 9 2 2}

21 14 0 3 3

22 7 2 1 12 3

J

^{?4 ?3 ?5 ?5 2 4 43 6 71 13 7 2 9 2 11 4 6 3 5 0}

?6

-

^{I+ 2 3 2}

J

^{?7 28} ?9 ⁸¹ 6 "38 ^{9 15} 21 l 0 ⁴ 6 27 6

.,o

31 7 16 5 8

-

^{12 10 20}

.1

^{11 2 45 103 4 5 20 Q}