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Science of the Total Environment

An International Journal for Scientific Research into the Environment and its Relationship with Humankind

Editor-in-Chief Executive Editor

J.O. Nriagu J.G. Farmer

Dept. of Environmental Health Sciences, School of GeoSciences, Crew Building,

School of Public Health, University of Michigan, University of Edinburgh,

109 S. Observatory Street, West Mains Road, Edinburgh, EH9 3JN,

Ann Arbor, MI 48109-2029, USA Scotland, UK

Tel.: +1 734 9360706; Fax: +1 734 6157141; Tel: +44 131 6504907; Fax: +44 131 6620478;

E-mail: stoten@umich.edu E-mail: stoten@ed.ac.uk

Associate Editors J.P. Bennett

University of Wisconsin, Institute for Environmental Studies, 445 Henry Mall, Madison WI 53706, USA

B.W. Brooks

Environmental Science and Biomedical Studies, Center for Reservoir and Aquatic Systems Research, Baylor University, One Bear Place #97266, Waco TX 76798-7266, USA

L. George

Portland State University, Environmental Sciences and Management, Portland OR 97201, USA

C.P. Huang

Department of Civil and Environmental Engineering, University of Delaware,

Newark, DE 19716 USA

A.B. MacKenzie

Scottish Universities Environmental Research Centre, Rankine Avenue, Scottish Enterprise Technology Park, East Kilbride G75 0QF, Scotland, UK

L. Morawska

School of Physical and Chemical Sciences, International Laboratory for Air Quality and Health Queensland University of Technology,

2 George Street, Brisbane, Q 4001 Australia Assistant Editor

M.C. Livingston

Department of Environmental Health Sciences, School of Public Health, University of Michigan, Ann Arbor, MI 48109-2029, USA

E-mail: stoten@umich.edu Editorial Board

S.J.T. Pollard Cranfield University, School of Applied Sciences, Cranfield, MK43 0AL, UK F. Rigét University of Aarhus, Dept. of Arctic Environment, Freder: Ksborgvej, 399, DK-4000 Roskilde, Denmark I. Snape Environmental Protection and Change Program, Australian Antarctic Division, Channel Highway, Kingston, Tasmania 7050 Australia C.E.W. Steinberg Institute of Biology, Freshwater Ecology, Humboldt University at Berlin, Arboretum, Spaethstr. 80/81, 12437 Berlin, Germany

Printed by Polestar Wheatons, Ltd., Exeter, UK The paper used in this publication meets the requirements of ANSI/NISO Z39.48-1992.

B. Ahman

Swed. Univ. of Agricultural Sciences R. Bargagli

Universita degli Studi di Sienna, Italy J. Burger

Rutgers University, Piscataway, USA N. Cape

Edinburgh Research Station, UK L. Chan

University of Northern British Columbia, Canada

M. Cresser

University of York, York, UK A. Cundy

University of Sussex, Brighton, UK J. Dorea

University of Brasilia, Brazil L.K. Duffy

University of Alaska, Fairbanks, USA X. Feng

Institute of Geochemistry, China A. Frank

Sweden University Agricultural Science/Clinical Chemistry/Veterinary Medicine, Uppsala, Sweden M.C. Graham

University of Edinburgh, Edinburgh, UK J.O. Grimalt

CID-CSIC, Barcelona, Spain

B.L. Gulson

Macquarie University, Sydney, Australia M. Gustin

University of Nevada, Reno, USA R.S. Hamilton

Middlesex University, London, UK P.T.C. Harrison

PTCH Consultancy Limited, Leicestershire, UK R.M. Harrison

University of Birmingham, UK P. Hooda

University of London, UK A.J. Horowitz

U.S. Geological Survey, Peachtree Business Center, Atlanta, USA K. Hudnell

105 Serrano Way, Chapel Hill, NC, USA D. Kolpin

U.S. Geological Survey, Iowa City, USA G. Lalor

University of the West Indies Mona, Jamaica X. Li

Hong Kong Polytechnic University, Hong Kong

L.Q. Ma

University of Florida, USA R.W. Macdonald

Institute of Ocean Sciences, Sidney, British Columbia, Canada

D. Muir

National Water Research Institute,

Environment Canada, Burlington ON, Canada M. Navarro-Alarcon

Department of Nutrition and Bromatology, University of Granada, Spain

M.L. Pignata

Universidad de Ciencias Exactas, Fisicas y Naturales, Argentina

L. Poissant

Environment Canada, Quebec, Canada C. Poschenrieder

Universidad Awconoma de Barcelona, Spain C. Reimann

Geological Survey of Norway, N–7491 Trondheim, Norway

E. Sabbioni

European Commission Joint Research Centre, Ispra, Italy

A. Smargiassi

Quebec National Institute for Public Health, Canada

S.H. Swan

Family and Community Medicine, Columbia, MO, USA

P. Szefer

Medical University of Gdansk, Poland F.M.G. Tack

Ghent University, Belgium J.-P. Weber

Toxicology Centre of the Quebec National Institute for Public Health, Canada

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