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Supplement of Atmos. Chem. Phys., 20, 13425–13441, 2020 https://doi.org/10.5194/acp-20-13425-2020-supplement

© Author(s) 2020. This work is distributed under the Creative Commons Attribution 4.0 License.

Supplement of

Atmospheric new particle formation characteristics in the Arctic as measured at Mount Zeppelin, Svalbard, from 2016 to 2018

Haebum Lee et al.

Correspondence to:Kihong Park (kpark@gist.ac.kr) and Young Jun Yoon (yjyoon@kopri.re.kr)

The copyright of individual parts of the supplement might differ from the CC BY 4.0 License.

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Figure S1. Comparison of monthly average size distributions obtained from the nano-SMPS (3–60 nm) and DMPS (10–810 nm) during the measurement period. The error bar indicates standard deviation.

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Figure S2. Monthly values of average chlorophyll-α concentration over the area (70–85º N, 25º W–50º E) and “air mass exposure to chlorophyll-α” (Echl) calculated by Eq. (1) in Park et al. (2018) from March to September during the measurement period.

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Figure S3. Relationship between N3–7 and J3–7 during NPF events with a liner regression line and a correction coefficient (r).

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Figure S4. Time series of (a) weekly N3–7, N7–25, NH3, and H2SO4, (b) daily GR and (c) daily J in different modes (J3–7, J7–25,

GR3–7, and GR7–25) during the measurement period.

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(a)

(b)

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Figure S5. Correlations of daily N3–25 versus (a) daily NH3, (b) daily SO2, and (c) daily H2SO4 concentrations during the measurement period. The dashed line represents a linear regression line with a correlation coefficient (r).

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Figure S6. NPF event probability distribution with daily CS and temperature. The cell size was 2 K (temperature) and the ratio of 1.26 between two consecutive CS values.

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Table S1. Average concentrations of ionic species (Na+, Mg2+, K+, NH4+, NO3, SO42–, and Cl) in particulate matter and gaseous species (NH3, SO2, and H2SO4) in different seasons during the measurement period.

Unit Spring Summer Fall Winter

Na+ μg m–3 0.27 ± 0.38 0.18 ± 0.28 0.22 ± 0.28 0.31 ± 0.33

Mg2+ μg m–3 0.04 ± 0.08 0.02 ± 0.04 0.03 ± 0.04 0.05 ± 0.05

K+ μg m–3 0.05 ± 0.07 0.03 ± 0.02 0.03 ± 0.02 0.03 ± 0.02

NH4+ μg N m–3 0.04 ± 0.05 0.02 ± 0.03 0.02 ± 0.03 0.02 ± 0.02

NO3 μg N m–3 0.02 ± 0.02 0.02 ± 0.02 0.02 ± 0.04 0.02 ± 0.02

SO42– μg S m–3 0.19 ± 0.18 0.08 ± 0.10 0.08 ± 0.09 0.11 ± 0.20

Cl μg m–3 0.39 ± 0.63 0.24 ± 0.43 0.35 ± 0.50 0.52 ± 0.59

NH3 μg N m–3 0.13 ± 0.60 0.16 ± 0.22 0.10 ± 0.10 0.08 ± 0.07

SO2 μg S m–3 0.09 ± 0.22 0.08 ± 0.11 0.08 ± 0.13 0.09 ± 0.27 H2SO4 105 molecules cm–3 7.43 ± 8.16 8.59 ± 8.64 5.52 ± 8.91 0.95 ± 0.69

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